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Solution-processed extremely thin films of Cu2SnS3 nanoparticles for planar heterojunction solar cells | |
Ashebir, Getinet Y.1,2; Dong, Chao1; Chen, Junwei1; Chen, Wangwei1,2; Liu, Rong1,2; Zhao, Qiuyuan1,2; Wan, Zhiyang1,2; Wang, Mingtai1 | |
2020-03-11 | |
发表期刊 | JOURNAL OF PHYSICS D-APPLIED PHYSICS |
ISSN | 0022-3727 |
通讯作者 | Dong, Chao(chaodone@126.com) ; Wang, Mingtai(mtwang@ipp.ac.cn) |
摘要 | Cu2SnS3 is a potential absorber material for thin film solar cells. However, Cu2SnS3 solar cells are normally prepared by high temperature sulfurization process. In this work, the Cu2SnS3 nanoparticle films with a porously structured surface are in situ prepared by a new and facile molecular precursor solution approach featuring a low annealing temperature (250 degrees C-350 degrees C) and a short annealing time (5 min); furthermore, the novel planar heterojunction solar cells configured as FTO/TiO2/CdS/Cu2SnS3/P3HT/MoO3/Ag are fabricated, in which poly(3-hexylthiophene) (P3HT), an organic conjugated polymer, mainly acts as hole transporting material. It is found that the annealing temperature imposes a significant influence on the structure of Cu2SnS3 nanoparticle film. While increasing annealing temperature leads to a higher crystallinity of Cu2SnS3 nanoparticle film, the pores on the film surface become larger at annealing temperature >300 degrees C. It is also revealed that the solar cell performance depends on the annealing temperature and Cu2SnS3 film thickness, and the efficiency of 2.03% is obtained in the solar cells with 60 nm thick Cu2SnS3 thin film prepared at 300 degrees C. The results here demonstrate a low-temperature solution preparation strategy to prepare Cu2SnS3 thin films for solar cells and other optoelectronic devices. |
关键词 | thin films Cu2SnS3 nanoparticles solar cells heterojunction |
DOI | 10.1088/1361-6463/ab5ee5 |
关键词[WOS] | LOW-COST ; CHEMICAL-SYNTHESIS ; CTS NANOPARTICLES ; EARTH-ABUNDANT ; QUANTUM DOTS ; ABSORBER ; TEMPERATURE ; CU2ZNSNS4 ; IMPACT ; LENGTH |
收录类别 | SCI |
语种 | 英语 |
资助项目 | National Natural Science Foundation of China[11274307] ; National Natural Science Foundation of China[91333121] ; National Natural Science Foundation of China[11474286] ; Science and Technology Project of Auhui Province[1604a0902148] ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology[2016FXZY003] |
项目资助者 | National Natural Science Foundation of China ; Science and Technology Project of Auhui Province ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology |
WOS研究方向 | Physics |
WOS类目 | Physics, Applied |
WOS记录号 | WOS:000519132200001 |
出版者 | IOP PUBLISHING LTD |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.hfcas.ac.cn:8080/handle/334002/103966 |
专题 | 中国科学院合肥物质科学研究院 |
通讯作者 | Dong, Chao; Wang, Mingtai |
作者单位 | 1.Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol, Hefei 230031, Peoples R China 2.Univ Sci & Technol China, Hefei 230026, Peoples R China |
推荐引用方式 GB/T 7714 | Ashebir, Getinet Y.,Dong, Chao,Chen, Junwei,et al. Solution-processed extremely thin films of Cu2SnS3 nanoparticles for planar heterojunction solar cells[J]. JOURNAL OF PHYSICS D-APPLIED PHYSICS,2020,53. |
APA | Ashebir, Getinet Y..,Dong, Chao.,Chen, Junwei.,Chen, Wangwei.,Liu, Rong.,...&Wang, Mingtai.(2020).Solution-processed extremely thin films of Cu2SnS3 nanoparticles for planar heterojunction solar cells.JOURNAL OF PHYSICS D-APPLIED PHYSICS,53. |
MLA | Ashebir, Getinet Y.,et al."Solution-processed extremely thin films of Cu2SnS3 nanoparticles for planar heterojunction solar cells".JOURNAL OF PHYSICS D-APPLIED PHYSICS 53(2020). |
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