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Three-wavelength measurement of aerosol absorption using a multi-resonator coupled photoacoustic spectrometer
Cao, Yuan1,2; Liu, Kun2; Wang, Ruifeng2; Chen, Weidong3; Gao, Xiaoming1,2
2021-01-18
发表期刊OPTICS EXPRESS
ISSN1094-4087
通讯作者Liu, Kun(liukun@aiofm.ac.cn) ; Gao, Xiaoming(xmgao@aiofm.ac.cn)
摘要Aerosol optical absorption measurements are important for the prediction of climate change, as aerosols directly disturb Earth's radiation balance by absorbing or scattering solar radiation. Although photoacoustic spectroscopy is commonly recognized as one of the best candidates to measure the absorption of aerosols, multi-wavelength measurements of aerosols optical absorption remain challenging. Here, a method based on photoacoustic spectroscopy that can simultaneously measure the aerosol absorption characteristics of three wavelengths (404, 637 and 805 nm) is proposed. In the three-wavelength photoacoustic spectrometer (TW-PAS), a photoacoustic cell with three acoustic resonators operating at different resonant frequencies was designed for offering multi-laser (multi-wavelength) operation simultaneously, and only one microphone was used to measure the acoustic signals of all resonators. The performance of TW-PAS was demonstrated and evaluated by measuring and analyzing the wavelength-dependent absorption coefficients of carbonaceous aerosols, which shows good agreement with previously reported results. The developed TW-PAS exhibits high potential for classifying and quantifying different types of light-absorbing aerosols by analyzing its absorption wavelength dependence characteristics. (C) 2021 Optical Society of America under the terms of the OSA Open Access Publishing Agreement
DOI10.1364/OE.412922
关键词[WOS]OPTICAL-PROPERTIES ; ANGSTROM EXPONENT ; LIGHT-ABSORPTION ; BROWN CARBON ; BLACK CARBON ; SCATTERING ; SPECTRA ; UV ; SPECTROSCOPY ; DEPENDENCE
收录类别SCI
语种英语
资助项目National Key Research and Development Program of China[2016YFC0303900] ; National Key Research and Development Program of China[2017YFC0209700] ; National Natural Science Foundation of China[41475023] ; National Natural Science Foundation of China[41575030] ; National Natural Science Foundation of China[41730103]
项目资助者National Key Research and Development Program of China ; National Natural Science Foundation of China
WOS研究方向Optics
WOS类目Optics
WOS记录号WOS:000609227300136
出版者OPTICAL SOC AMER
引用统计
被引频次:17[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.hfcas.ac.cn:8080/handle/334002/119846
专题中国科学院合肥物质科学研究院
通讯作者Liu, Kun; Gao, Xiaoming
作者单位1.Univ Sci & Technol China, Sch Environm Sci & Optoelect Technol, Hefei 230031, Peoples R China
2.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Hefei 230031, Peoples R China
3.Univ Littoral Cote dOpale, Lab Phys Chim Atmosphere, 189A,Av Maurice Schumann, F-59140 Dunkerque, France
第一作者单位中科院安徽光学精密机械研究所
通讯作者单位中科院安徽光学精密机械研究所
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GB/T 7714
Cao, Yuan,Liu, Kun,Wang, Ruifeng,et al. Three-wavelength measurement of aerosol absorption using a multi-resonator coupled photoacoustic spectrometer[J]. OPTICS EXPRESS,2021,29.
APA Cao, Yuan,Liu, Kun,Wang, Ruifeng,Chen, Weidong,&Gao, Xiaoming.(2021).Three-wavelength measurement of aerosol absorption using a multi-resonator coupled photoacoustic spectrometer.OPTICS EXPRESS,29.
MLA Cao, Yuan,et al."Three-wavelength measurement of aerosol absorption using a multi-resonator coupled photoacoustic spectrometer".OPTICS EXPRESS 29(2021).
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