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Converting Co2+-impregnated g-C3N4 into N-doped CNTs-confined Co nanoparticles for efficient hydrogenation rearrangement reactions of furanic aldehydes
Wang, Dongdong1,2; Al-Mamun, Mohammad3; Gong, Wanbing1; Lv, Yang1,2; Chen, Chun1; Lin, Yue4; Wang, Guozhong1; Zhang, Haimin1; Zhao, Huijun1,3
2021-01-05
Source PublicationNANO RESEARCH
ISSN1998-0124
Corresponding AuthorGong, Wanbing(wbgong@issp.ac.cn) ; Zhao, Huijun(h.zhao@griffith.edu.au)
AbstractThe cyclopentanone and derivatives are a class of crucial fine chemicals for various industries and currently produced by conventional petrochemical synthetic routes. Here, we demonstrated a new synthetic approach to directly fabricate N-doped carbon nanotube (N-CNTs) networks with confined Co nanoparticles from Co2+-impregnated bulk g-C3N4 as high performance hydrogenation rearrangement (HR) catalyst to efficiently convert a wide spectrum of biomass-derived furanic aldehydes to the corresponding cyclopentanones in water under a record-low H-2 pressure of 0.5 MPa and mild temperature. We unveiled a Co-catalysed bulk g-C3N4 decomposition/carbonisation CNTs formation mechanism. A new HR pathway was also unveiled.
Keywordg-C3N4 Co nanoparticles carbon nanotubes hydrogenation rearrangement furanic aldehydes
DOI10.1007/s12274-021-3298-y
WOS KeywordSELECTIVE HYDROGENATION ; CARBON NANOTUBES ; CYCLOPENTANONE ; CATALYSTS ; CONVERSION ; PERFORMANCE ; HYBRIDS ; BOND
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[51871209] ; National Natural Science Foundation of China[51902311] ; Postdoctoral Science Foundation of China[2019M652223]
Funding OrganizationNational Natural Science Foundation of China ; Postdoctoral Science Foundation of China
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS SubjectChemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied
WOS IDWOS:000605145200005
PublisherTSINGHUA UNIV PRESS
Citation statistics
Document Type期刊论文
Identifierhttp://ir.hfcas.ac.cn:8080/handle/334002/119963
Collection中国科学院合肥物质科学研究院
Corresponding AuthorGong, Wanbing; Zhao, Huijun
Affiliation1.Chinese Acad Sci, Anhui Key Lab Nanomat & Nanotechnol, CAS Ctr Excellence Nanosci,Key Lab Mat Phys, Inst Solid State Phys,Ctr Environm & Energy Nanom, Hefei 230031, Peoples R China
2.Univ Sci & Technol China, Hefei 230026, Peoples R China
3.Griffith Univ, Ctr Clean Environm & Energy, Gold Coast Campus, Brisbane, Qld 4222, Australia
4.Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Peoples R China
Recommended Citation
GB/T 7714
Wang, Dongdong,Al-Mamun, Mohammad,Gong, Wanbing,et al. Converting Co2+-impregnated g-C3N4 into N-doped CNTs-confined Co nanoparticles for efficient hydrogenation rearrangement reactions of furanic aldehydes[J]. NANO RESEARCH,2021.
APA Wang, Dongdong.,Al-Mamun, Mohammad.,Gong, Wanbing.,Lv, Yang.,Chen, Chun.,...&Zhao, Huijun.(2021).Converting Co2+-impregnated g-C3N4 into N-doped CNTs-confined Co nanoparticles for efficient hydrogenation rearrangement reactions of furanic aldehydes.NANO RESEARCH.
MLA Wang, Dongdong,et al."Converting Co2+-impregnated g-C3N4 into N-doped CNTs-confined Co nanoparticles for efficient hydrogenation rearrangement reactions of furanic aldehydes".NANO RESEARCH (2021).
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