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Evaluating the electro-sensing behaviors of single-atom catalysts based on mechanistic insights
Lin, Chu-Hong; Yang, Meng; Li, Pei-Hua; Huang, Xing-Jiu
2021-02-01
Source PublicationCURRENT OPINION IN ELECTROCHEMISTRY
ISSN2451-9103
Corresponding AuthorLin, Chu-Hong(chlin@iim.ac.cn) ; Huang, Xing-Jiu(xingjiuhuang@iim.ac.cn)
AbstractSingle-atom catalysts (SACs) have been widely applied as electrocatalysts due to their excellent catalytic ability, selectivity, and stability, which are also key aspects considered for electro-sensing interfaces. Typical SACs are catalytic single atoms dispersed over oxide-, sulfide-, or carbon-based material supports. In this review, the electrocatalytic mechanisms of SACs are briefly summarized. SACs can increase the reactivity and modulate the reaction pathway via redox mediating, adsorbing to the preferred reactant/intermediate, and cooperating with other active sites either from the substrate or from a nearby heteroatom. Based on the mechanistic insights of SACs, this review aims to provide some inspirations for future applications of SACs in the design of efficient electro-sensing interfaces.
KeywordSingle atom catalysts Catalytic mechanism Redox mediator Adsorption Synergistic effect Electro-sensing
DOI10.1016/j.coelec.2020.100646
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[21802145] ; National Natural Science Foundation of China[21735005] ; Natural Science Foundation of Anhui Province[2008085QB79] ; One Hundred Person Project, Chinese Academy of Sciences, China
Funding OrganizationNational Natural Science Foundation of China ; Natural Science Foundation of Anhui Province ; One Hundred Person Project, Chinese Academy of Sciences, China
WOS Research AreaChemistry ; Electrochemistry ; Materials Science
WOS SubjectChemistry, Physical ; Electrochemistry ; Materials Science, Multidisciplinary
WOS IDWOS:000632820800023
PublisherELSEVIER
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Document Type期刊论文
Identifierhttp://ir.hfcas.ac.cn:8080/handle/334002/121802
Collection中国科学院合肥物质科学研究院
Corresponding AuthorLin, Chu-Hong; Huang, Xing-Jiu
AffiliationChinese Acad Sci, Environm Mat & Pollut Control Lab, Inst Solid State Phys, HFIPS, Hefei 230031, Peoples R China
Recommended Citation
GB/T 7714
Lin, Chu-Hong,Yang, Meng,Li, Pei-Hua,et al. Evaluating the electro-sensing behaviors of single-atom catalysts based on mechanistic insights[J]. CURRENT OPINION IN ELECTROCHEMISTRY,2021,25.
APA Lin, Chu-Hong,Yang, Meng,Li, Pei-Hua,&Huang, Xing-Jiu.(2021).Evaluating the electro-sensing behaviors of single-atom catalysts based on mechanistic insights.CURRENT OPINION IN ELECTROCHEMISTRY,25.
MLA Lin, Chu-Hong,et al."Evaluating the electro-sensing behaviors of single-atom catalysts based on mechanistic insights".CURRENT OPINION IN ELECTROCHEMISTRY 25(2021).
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