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Epitaxial growth and room-temperature ferromagnetism of quasi-2D layered Cr4Te5 thin film
Wang, Jing1; Wang, Weiyuan1; Fan, Jiyu1,2; Zheng, Huan1; Liu, Hao1; Ma, Chunlan3; Zhang, Lei4; Tong, Wei4; Ling, Langsheng4; Zhu, Yan1,2; Yang, Hao1,2
2022-04-21
发表期刊JOURNAL OF PHYSICS D-APPLIED PHYSICS
ISSN0022-3727
通讯作者Fan, Jiyu(jiyufan@nuaa.edu.cn) ; Yang, Hao(yanghao@nuaa.edu.cn)
摘要Large-scale growth of two-dimensional (2D) ferromagnetic thin films will provide an ideal platform for studying 2D magnetism and active spintronic devices. However, controllable growth of 2D ferromagnets over large areas faces tremendous challenges. Herein, we report a large-area growth of 2D ferromagnetic single-crystal thin films Cr4Te5 on Al2O3 (0001) substrates using pulsed laser deposition. X-ray diffraction patterns and atomic force microscopy detection confirm that all thin films have high quality epitaxy together with being atom-level smooth. Magnetic measurements show the persistence of ferromagnetic ordering state to above room temperature, with a Curie temperature similar to 320 K, atomic magnetic moment similar to 0.307 mu(B)/Cr, and the easy-magnetization axis in the film plane. Comparing with bulk Cr4Te5 single-crystal, the critical exponent beta = 0.491 indicates that the magnetic interactions of the thin film obey the mean-field model rather than the 3D Heisenberg model. This work will open an avenue for growing large-scale 2D ferromagnets and developing room temperature 2D magnet-based nanodevices.
关键词van der Waals magnet epitaxial film 2D material Cr4Te5
DOI10.1088/1361-6463/ac47c2
关键词[WOS]MAGNETIC-PROPERTIES ; CR3TE4 ; CR2TE3 ; CRTE ; TE ; SE
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China[11974181] ; National Natural Science Foundation of China[11774172] ; Top-notch Academic Programs Project of Jiangsu Higher Education Institutions (TAPP)
项目资助者National Natural Science Foundation of China ; Top-notch Academic Programs Project of Jiangsu Higher Education Institutions (TAPP)
WOS研究方向Physics
WOS类目Physics, Applied
WOS记录号WOS:000746166700001
出版者IOP Publishing Ltd
引用统计
被引频次:4[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.hfcas.ac.cn:8080/handle/334002/127348
专题中国科学院合肥物质科学研究院
通讯作者Fan, Jiyu; Yang, Hao
作者单位1.Nanjing Univ Aeronaut & Astronaut, Dept Appl Phys, Nanjing 210016, Peoples R China
2.MILT, Key Lab Aerosp Informat Mat & Phys NUAA, Nanjing 211106, Peoples R China
3.Suzhou Univ Sci & Technol, Sch Phys Sci & Technol, Jiangsu Key Lab Micro & Nano Heat Fluid Flow Tech, Suzhou 215009, Peoples R China
4.Chinese Acad Sci, Anhui Key Lab Condensed Matter Phys Extreme Condi, High Magnet Field Lab, Hefei 230031, Peoples R China
推荐引用方式
GB/T 7714
Wang, Jing,Wang, Weiyuan,Fan, Jiyu,et al. Epitaxial growth and room-temperature ferromagnetism of quasi-2D layered Cr4Te5 thin film[J]. JOURNAL OF PHYSICS D-APPLIED PHYSICS,2022,55.
APA Wang, Jing.,Wang, Weiyuan.,Fan, Jiyu.,Zheng, Huan.,Liu, Hao.,...&Yang, Hao.(2022).Epitaxial growth and room-temperature ferromagnetism of quasi-2D layered Cr4Te5 thin film.JOURNAL OF PHYSICS D-APPLIED PHYSICS,55.
MLA Wang, Jing,et al."Epitaxial growth and room-temperature ferromagnetism of quasi-2D layered Cr4Te5 thin film".JOURNAL OF PHYSICS D-APPLIED PHYSICS 55(2022).
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