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Pressure-induced superconductivity in quasi-one-dimensional semimetal Ta2PdSe6 | |
Yang, Haiyang1,2; Zhou, Yonghui1![]() ![]() ![]() ![]() ![]() ![]() | |
2022-08-17 | |
发表期刊 | PHYSICAL REVIEW MATERIALS
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ISSN | 2475-9953 |
通讯作者 | Zhou, Yonghui(yhzhou@hmfl.ac.cn) ; Yang, Xiaoping(xpyang@hmfl.ac.cn) ; Yang, Zhaoron(zryang@issp.ac.cn) |
摘要 | Here we report the discovery of pressure-induced superconductivity in quasi-one-dimensional Ta2PdSe6, through a combination of electrical transport, synchrotron x-ray diffraction, and theoretical calculations. Our transport measurements show that the superconductivity appears at a critical pressure P-c similar to 18.3 GPa and is robust upon further compression up to 62.6 GPa. The estimated upper critical field mu H-0(c2)(0) in the pressurized Ta2PdSe6 is much lower than the Pauli limiting field, in contrast to the case in its isostructural analogs M2PdxX5 (M = Nb, Ta; X = S, Se). Concomitant with the occurrence of superconductivity, anomalies in pressure-dependent transport properties are observed, including sign reversal of Hall coefficient, abnormally enhanced resistance, and dramatically suppressed magnetoresistance. Meanwhile, room-temperature synchrotron x-ray diffraction experiments reveal the stability of the pristine monoclinic structure (space group C2/m) upon compression. Combined with the density functional theory calculations, we argue that a pressure-induced Lifshitz transition could be the electronic origin of the emergent superconductivity in Ta2PdSc6. |
DOI | 10.1103/PhysRevMaterials.6.084803 |
关键词[WOS] | TRANSITION ; METAL |
收录类别 | SCI |
语种 | 英语 |
资助项目 | National Key Research and Development Program of China[2018YFA0305700] ; National Key Research and Development Program of China[2021YFA1600204] ; National Natural Science Foundation of China[U1932152] ; National Natural Science Foundation of China[11874362] ; National Natural Science Foundation of China[12174395] ; National Natural Science Foundation of China[12004004] ; National Natural Science Foundation of China[11704387] ; National Natural Science Foundation of China[U19A2093] ; National Natural Science Foundation of China[U1832209] ; National Natural Science Foundation of China[12174397] ; Natural Science Foundation of Anhui Province[1808085MA06] ; Natural Science Foundation of Anhui Province[2008085QA40] ; Natural Science Foundation of Anhui Province[1908085QA18] ; Users with Excellence Project of Hefei Center CAS[2021HSC-UE008] ; Users with Excellence Project of Hefei Center CAS[2020HSC-UE015] ; Collaborative Innovation Program of Hefei Science Center CAS[2020HSC-CIP014] ; High Magnetic Field Laboratory of Anhui Province[AHHM-FX-2020-02] ; High Magnetic Field Laboratory of Anhui Province[AHHM-FX-2021-03] ; Youth Innovation Promotion Association CAS[2020443] |
项目资助者 | National Key Research and Development Program of China ; National Natural Science Foundation of China ; Natural Science Foundation of Anhui Province ; Users with Excellence Project of Hefei Center CAS ; Collaborative Innovation Program of Hefei Science Center CAS ; High Magnetic Field Laboratory of Anhui Province ; Youth Innovation Promotion Association CAS |
WOS研究方向 | Materials Science |
WOS类目 | Materials Science, Multidisciplinary |
WOS记录号 | WOS:000844399900001 |
出版者 | AMER PHYSICAL SOC |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.hfcas.ac.cn:8080/handle/334002/132030 |
专题 | 中国科学院合肥物质科学研究院 |
通讯作者 | Zhou, Yonghui; Yang, Xiaoping; Yang, Zhaoron |
作者单位 | 1.Chinese Acad Sci, Anhui Key Lab Condensed Matter Phys Extreme Condit, High Magnet Field Lab, HFIPS, Hefei 230031, Peoples R China 2.Univ Sci & Technol China, Sci Isl Branch, Grad Sch, Hefei 230026, Peoples R China 3.Anhui Univ, Inst Phys Sci & Informat Technol, Hefei 230601, Peoples R China 4.Chinese Acad Sci, Shanghai Adv Res Inst, Shanghai Synchrotron Radiat Facil, Shanghai 201204, Peoples R China |
推荐引用方式 GB/T 7714 | Yang, Haiyang,Zhou, Yonghui,Li, Liangyu,et al. Pressure-induced superconductivity in quasi-one-dimensional semimetal Ta2PdSe6[J]. PHYSICAL REVIEW MATERIALS,2022,6. |
APA | Yang, Haiyang.,Zhou, Yonghui.,Li, Liangyu.,Chen, Zheng.,Zhang, Zhuyi.,...&Yang, Zhaoron.(2022).Pressure-induced superconductivity in quasi-one-dimensional semimetal Ta2PdSe6.PHYSICAL REVIEW MATERIALS,6. |
MLA | Yang, Haiyang,et al."Pressure-induced superconductivity in quasi-one-dimensional semimetal Ta2PdSe6".PHYSICAL REVIEW MATERIALS 6(2022). |
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