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Graphene oxides with different oxidation degrees for Co(II) ion pollution management
Liu, Xia1; Huang, Yongshun1; Duan, Shengxia1; Wang, Yanan1; Li, Jiaxing1,3,4; Chen, Yuantao2; Hayat, Tasawar4,5; Wang, Xiangke3,4
2016-10-15
发表期刊CHEMICAL ENGINEERING JOURNAL
摘要Presented herein is a facile approach, which is easy, cost-effective, environmental benign without any secondary environmental pollution and no requirement for post purification, towards the synthesis of graphene oxides (GOs) with different oxidation degrees by ozone treatment. The synthesized GOs with controlled oxidation degrees can not only increase the quantity of oxygen-containing functional groups on GOs surfaces, but also decrease the sizes of GOs sheets to facilitate their dispersion abilities in aqueous solution, as revealed by characterization. The ozonized GOs were further applied as Co(II) adsorbents from aqueous solutions. The adsorption results showed that this adsorption processes was endothermic and spontaneous, and followed the pseudo-second-order kinetics and the Langmuir adsorption models. The microcosmic mechanism displayed that cobalt can complex with the oxygen-containing functional groups on GOs surfaces. As expected, increased adsorption capacities were observed by GOS with higher oxidation degrees. (C) 2016 Elsevier B.V. All rights reserved.
文章类型Article
关键词Ozone Oxidation Graphene Oxides Co(Ii) Adsorption
WOS标题词Science & Technology ; Technology
DOI10.1016/j.cej.2016.05.107
关键词[WOS]LAYERED DOUBLE HYDROXIDE ; AQUEOUS-SOLUTION ; ENHANCED SEQUESTRATION ; METAL-IONS ; ADSORPTION ; REMOVAL ; NANOSHEETS ; COBALT ; KINETICS ; EXCHANGE
收录类别SCI
语种英语
项目资助者National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; National Natural Science Foundation of China(21272236) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Chinese National Fusion Project for ITER(2013GB110005) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Special Scientific Research Fund of Public Welfare Profession of China(201509074) ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Kunlun Scholarship of Qinghai Province ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Jiangsu Provincial Key Laboratory of Radiation Medicine and Protection ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions
WOS研究方向Engineering
WOS类目Engineering, Environmental ; Engineering, Chemical
WOS记录号WOS:000382590900078
引用统计
被引频次:64[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.hfcas.ac.cn:8080/handle/334002/21428
专题中科院等离子体物理研究所
作者单位1.Chinese Acad Sci, Inst Plasma Phys, Key Lab Novel Thin Film Solar Cells, POB 1126, Hefei 230031, Peoples R China
2.Qinghai Normal Univ, Dept Chem, Xining 810008, Qinghai, Peoples R China
3.Collaborat Innovat Ctr Radiat Med Jiangsu Higher, Suzhou, Jiangsu, Peoples R China
4.King Abdulaziz Univ, NAAM Res Grp, Fac Sci, Jeddah 21589, Saudi Arabia
5.Quaid I Azam Univ, Dept Math, Islamabad 44000, Pakistan
第一作者单位中科院等离子体物理研究所
推荐引用方式
GB/T 7714
Liu, Xia,Huang, Yongshun,Duan, Shengxia,et al. Graphene oxides with different oxidation degrees for Co(II) ion pollution management[J]. CHEMICAL ENGINEERING JOURNAL,2016,302(无):763-772.
APA Liu, Xia.,Huang, Yongshun.,Duan, Shengxia.,Wang, Yanan.,Li, Jiaxing.,...&Wang, Xiangke.(2016).Graphene oxides with different oxidation degrees for Co(II) ion pollution management.CHEMICAL ENGINEERING JOURNAL,302(无),763-772.
MLA Liu, Xia,et al."Graphene oxides with different oxidation degrees for Co(II) ion pollution management".CHEMICAL ENGINEERING JOURNAL 302.无(2016):763-772.
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