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Experimental and theoretical studies on competitive adsorption of aromatic compounds on reduced graphene oxides
Yu, Shujun1,2; Wang, Xiangxue1,2; Ai, Yuejie1; Tan, Xiaoli2,3; Hayat, Tasawar4,5; Hu, Wenping6; Wang, Xiangke1,3,5
2016
Source PublicationJOURNAL OF MATERIALS CHEMISTRY A
AbstractThe individual and competitive adsorption studies of benzene, aniline and naphthylamine on reduced graphene oxides (rGOs) were investigated by batch experiments and theoretical density functional theory (DFT). Experimental results indicate that (1) in all the single, binary, and ternary aromatic compound systems, the sequence of maximum adsorption capacity is naphthylamine > aniline > benzene on rGOs; (2) the overall adsorption capacity of rGOs is in the order of ternary > binary > single system. The DFT calculations indicate that (1) the adsorption energy (E-ad) follows the order of E-ad (benzene) < E-ad (aniline) < E-ad (naphthylamine); (2) the binding energy (Ebd) values of aromatic mixtures indicate that the intramolecular interactions between the aromatic compounds themselves have an important influence on their adsorption on rGOs. The DFT calculations are in good agreement with the batch adsorption results. These findings are very important and useful to understand the mechanisms of adsorption of aromatic compounds on rGOs as well as assessing the effect of the benzene-ring number and polar functional groups on the adsorption of coexisting aromatic compounds on rGOs. The contents are important for the application of rGOs in environmental pollution management.
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
DOI10.1039/c6ta00890a
WOS KeywordMULTIWALLED CARBON NANOTUBES ; DENSITY-FUNCTIONAL THERMOCHEMISTRY ; ACTIVATED CARBON ; HIGHLY EFFICIENT ; RAMAN-SPECTROSCOPY ; GRAPHITE OXIDE ; EXACT-EXCHANGE ; BISPHENOL-A ; HUMIC-ACID ; NANOSHEETS
Indexed BySCI
Language英语
Funding OrganizationNational Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; National Natural Science Foundation of China(21577032 ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Priority Academic Program Development of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education Institutions ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Deanship of Scientific Research (DSR), King Abdulaziz University(41-130-36-HiCi) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; Fundamental Research Funds for the Central Universities(JB2015001) ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 21225730 ; 91326202 ; 91326202 ; 91326202 ; 91326202 ; 91326202 ; 91326202 ; 91326202 ; 91326202 ; 91326202 ; 91326202 ; 91326202 ; 91326202 ; 91326202 ; 91326202 ; 91326202 ; 91326202 ; 21207135 ; 21207135 ; 21207135 ; 21207135 ; 21207135 ; 21207135 ; 21207135 ; 21207135 ; 21207135 ; 21207135 ; 21207135 ; 21207135 ; 21207135 ; 21207135 ; 21207135 ; 21207135 ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134)
WOS Research AreaChemistry ; Energy & Fuels ; Materials Science
WOS SubjectChemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary
WOS IDWOS:000374790400035
Citation statistics
Cited Times:132[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.hfcas.ac.cn:8080/handle/334002/21761
Collection中科院等离子体物理研究所
Affiliation1.North China Elect Power Univ, Sch Environm & Chem Engn, Beijing 102206, Peoples R China
2.Chinese Acad Sci, Inst Plasma Phys, Key Lab Novel Thin Film Solar Cells, Hefei 230031, Peoples R China
3.Soochow Univ, Sch Radiol & Interdisciplinary Sci, Collaborat Innovat Ctr Radiat Med Jiangsu Higher, Suzhou 215123, Peoples R China
4.Quaid I Azam Univ, Dept Math, Islamabad 44000, Pakistan
5.King Abdulaziz Univ, NAAM Res Grp, Fac Sci, Jeddah 21589, Saudi Arabia
6.Chinese Acad Sci, Inst Chem, Key Lab Organ Solids, Beijing 100190, Peoples R China
First Author AffilicationChinese Academy of Sciences, Institute of Plasma Physics, Hefei 230031, Anhui, Peoples R China
Recommended Citation
GB/T 7714
Yu, Shujun,Wang, Xiangxue,Ai, Yuejie,et al. Experimental and theoretical studies on competitive adsorption of aromatic compounds on reduced graphene oxides[J]. JOURNAL OF MATERIALS CHEMISTRY A,2016,4(15):5654-5662.
APA Yu, Shujun.,Wang, Xiangxue.,Ai, Yuejie.,Tan, Xiaoli.,Hayat, Tasawar.,...&Wang, Xiangke.(2016).Experimental and theoretical studies on competitive adsorption of aromatic compounds on reduced graphene oxides.JOURNAL OF MATERIALS CHEMISTRY A,4(15),5654-5662.
MLA Yu, Shujun,et al."Experimental and theoretical studies on competitive adsorption of aromatic compounds on reduced graphene oxides".JOURNAL OF MATERIALS CHEMISTRY A 4.15(2016):5654-5662.
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