Institutional Repository of Chinese Academy of Sciences, Institute of Plasma Physics, Hefei 230031, Anhui, Peoples R China
Facile preparation of amino functionalized graphene oxide decorated with Fe3O4 nanoparticles for the adsorption of Cr(VI) | |
Zhao, Donglin1; Gao, Xuan1; Wu, Changnian1; Xie, Rong1; Feng, Shaojie1; Chen, Changlun2![]() | |
2016-10-30 | |
发表期刊 | APPLIED SURFACE SCIENCE
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摘要 | A novel ternary magnetic composite consisting of graphene oxide (GO), diethylenetriamine and Fe3O4 nanoparticles (AMGO) were synthesized by a facile one-step reaction route and characterized. The AMGO was applied as a magnetic adsorbent for the Cr(VI) removal from aqueous solutions and the magnetic separation process only took 40 s. The maximum adsorption capacity of the AMGO for Cr(VI) was 123.4 mg/g, displaying a high efficiency for the removal of Cr(VI), which was much higher than that of MGO. The removal process was pH dependence, endothermic and spontaneous. The pseudo-second-order model described well the adsorption kinetic data and the Langmuir isotherm model fitted the experimental data better than the Freundlich isotherm model. XPS analysis revealed that the Cr(VI) was reduced to the low-toxicity Cr(III) during the adsorption process. Both the Cr(VI) adsorption and subsequent reduction of adsorbed Cr(VI) to Cr(III) contributed to the Cr(VI) removal. In addition, the excellent reproducibility indicate that the AMGO may be a promising adsorption material for the separation and preconcentration of Cr(VI) ions from aqueous solutions in environmental pollution cleanup. (C) 2016 Elsevier B.V. All rights reserved. |
文章类型 | Article |
关键词 | Fe3o4/graphene Oxide Composite Adsorption Cr(Vi) |
WOS标题词 | Science & Technology ; Physical Sciences ; Technology |
DOI | 10.1016/j.apsusc.2016.05.022 |
关键词[WOS] | ZERO-VALENT IRON ; FAST CHROMIUM REMOVAL ; AQUEOUS-SOLUTION ; MAGNETIC CYCLODEXTRIN ; ACTIVATED CARBON ; WASTE-WATER ; HEAVY-METAL ; NANOCOMPOSITE ; COMPOSITES ; NANOSHEETS |
收录类别 | SCI |
语种 | 英语 |
项目资助者 | National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; National Natural Science Foundation of China(21377005 ; 21477133 ; 21477133 ; 21477133 ; 21477133 ; 21477133 ; 21477133 ; 21477133 ; 21477133 ; 21477133 ; 21477133 ; 21477133 ; 21477133 ; 21477133 ; 21477133 ; 21477133 ; 21477133 ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) ; 41273134) |
WOS研究方向 | Chemistry ; Materials Science ; Physics |
WOS类目 | Chemistry, Physical ; Materials Science, Coatings & Films ; Physics, Applied ; Physics, Condensed Matter |
WOS记录号 | WOS:000378560900001 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.hfcas.ac.cn:8080/handle/334002/21766 |
专题 | 中科院等离子体物理研究所 |
作者单位 | 1.Anhui Jianzhu Univ, Key Lab Funct Mol Design & Interface Proc, Hefei 230601, Peoples R China 2.Chinese Acad Sci, Inst Plasma Phys, POB 1126, Hefei 230031, Peoples R China |
推荐引用方式 GB/T 7714 | Zhao, Donglin,Gao, Xuan,Wu, Changnian,et al. Facile preparation of amino functionalized graphene oxide decorated with Fe3O4 nanoparticles for the adsorption of Cr(VI)[J]. APPLIED SURFACE SCIENCE,2016,384(无):1-9. |
APA | Zhao, Donglin,Gao, Xuan,Wu, Changnian,Xie, Rong,Feng, Shaojie,&Chen, Changlun.(2016).Facile preparation of amino functionalized graphene oxide decorated with Fe3O4 nanoparticles for the adsorption of Cr(VI).APPLIED SURFACE SCIENCE,384(无),1-9. |
MLA | Zhao, Donglin,et al."Facile preparation of amino functionalized graphene oxide decorated with Fe3O4 nanoparticles for the adsorption of Cr(VI)".APPLIED SURFACE SCIENCE 384.无(2016):1-9. |
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