Institutional Repository of Key Laboratory of Ion Beam Bioengineering, Hefei Institutes of Physical Science, Chinese Academy of Sciences, Hefei, Anhui 230031, People's Republic of China
Adsorption of methylene blue from aqueous solution onto multiporous palygorskite modified by ion beam bombardment: Effect of contact time, temperature, pH and ionic strength | |
Zhang, Jing1; Cai, Dongqing1; Zhang, Guilong1; Cai, Chuanjie1; Zhang, Caili1; Qiu, Guannan1; Zheng, Kang2; Wu, Zhengyan1 | |
2013-10-01 | |
发表期刊 | APPLIED CLAY SCIENCE |
摘要 | Our previous work has reported that an inorganic nano-network of palygorskite with multiporous structure can be fabricated from rigid nano-rods by ion beam bombardment and has better adsorption capability than nanorods. Here, this dispersed modified nano adsorbent was characterized by Fourier Transform Infrared (FTIR) spectroscopy and Scanning Electron Microscope (SEM). The adsorption property of methylene blue (MB) onto this adsorbent was investigated. It was found that the adsorption capacity increased with contact time, pH, MB initial concentration, respectively, and then reached an equilibrium. Moreover, the effect of pH on the adsorption was strongly determined by zeta potential. The adsorption kinetics of MB was dominated by the pseudo-secondorder reaction model, and the adsorption isotherms fit the Freundlich isotherms better than the Langmuir isotherms. Three temperatures (293 K, 303 K, 313 K) were set for describing the thermodynamic parameters (Delta H-theta, Delta S-theta, Delta G(theta)), which indicated that the adsorption was spontaneous and exothermic. Lastly, the mechanism of the influence of ionic strength on the adsorption was discussed. (C) 2013 Elsevier B.V. All rights reserved. |
文章类型 | Article |
关键词 | Palygorskite Ion Beam Bombardment Methylene Blue Adsorption |
WOS标题词 | Science & Technology ; Physical Sciences ; Technology |
DOI | 10.1016/j.clay.2013.08.033 |
关键词[WOS] | FIXED-BED COLUMN ; ACTIVATED CARBON ; REACTIVE DYE ; SORPTION ; REMOVAL ; EQUILIBRIUM ; BENTONITE ; CHITOSAN ; KINETICS ; BIOMASS |
收录类别 | SCI |
语种 | 英语 |
WOS研究方向 | Chemistry ; Materials Science ; Mineralogy |
WOS类目 | Chemistry, Physical ; Materials Science, Multidisciplinary ; Mineralogy |
WOS记录号 | WOS:000326661300019 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.hfcas.ac.cn:8080/handle/334002/22185 |
专题 | 技术生物与农业工程研究所 |
作者单位 | 1.Chinese Acad Sci, Hefei Inst Phys Sci, Key Lab Ion Beam Bioengn, Hefei 230031, Peoples R China 2.Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Jing,Cai, Dongqing,Zhang, Guilong,et al. Adsorption of methylene blue from aqueous solution onto multiporous palygorskite modified by ion beam bombardment: Effect of contact time, temperature, pH and ionic strength[J]. APPLIED CLAY SCIENCE,2013,83-84:137-143. |
APA | Zhang, Jing.,Cai, Dongqing.,Zhang, Guilong.,Cai, Chuanjie.,Zhang, Caili.,...&Wu, Zhengyan.(2013).Adsorption of methylene blue from aqueous solution onto multiporous palygorskite modified by ion beam bombardment: Effect of contact time, temperature, pH and ionic strength.APPLIED CLAY SCIENCE,83-84,137-143. |
MLA | Zhang, Jing,et al."Adsorption of methylene blue from aqueous solution onto multiporous palygorskite modified by ion beam bombardment: Effect of contact time, temperature, pH and ionic strength".APPLIED CLAY SCIENCE 83-84(2013):137-143. |
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