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The influence of biochar type on long-term stabilization for Cd and Cu in contaminated paddy soils
Li, Hongying1,2; Ye, Xinxin1; Geng, Zhigang1; Zhou, Hongjian1; Guo, Xisheng2; Zhang, Yunxia1; Zhao, Huijun1,3; Wang, Guozhong1
2016-03-05
发表期刊JOURNAL OF HAZARDOUS MATERIALS
摘要Long-term effect of biochar on PTEs (potential toxic elements) immobilization depends upon biochar own property and its aging process in soil. To understand the role of biachar type on PTEs stabilization, two types of biochar, corn-straw-derived biochar (CB) and hardwood-derived biochar (HB), were compared for their efficacy in achieving a stable decrease in the bio-availability of Cd and Cu in soils. The 3-year pot-culture experiment showed that HB reduced the concentration of CaCl2-extractable Cd and Cu by 57.9 and 63.8% in soil, and Cd and Cu uptake by 63.6 and 56.3% in rice tissue respectively, in the first year, whereas these values increased in the next two years. On the other hand, CB decreased these values steadily year by year. At the end of the 3 years, CB at 5% level had lowered the levels of CaCl2-extractable Cd and Cu by 53.6 and 66.8%, respectively. These variations between CB and HB were due to the differences in the way the two types of biochar age in the soil. The aging process was simulated in the laboratory, and the XPS results showed that the oxidization of the biochars introduced more oxygen-containing groups (especially carboxyl) on the surface of CB than HB, leading to a correspondingly greater number of oxygenated binding sites for Cd and Cu in the case of CB. The content of lignin was the major factor resulting in the variation of oxidation degree in two biochars. These results suggest that it is important to select the right kind of biochar to stably decrease the bio-availability of potential toxic elements (Cd and Cu) in contaminated soils. (C) 2015 Elsevier B.V. All rights reserved.
文章类型Article
关键词Rice Soil Remediation Biochar Acid Soil Bio-availability
WOS标题词Science & Technology ; Technology ; Life Sciences & Biomedicine
DOI10.1016/j.jhazmat.2015.10.048
关键词[WOS]STRAW DERIVED BIOCHAR ; HEAVY-METALS ; GREENWASTE COMPOST ; ACTIVATED CARBONS ; FUNCTIONAL-GROUPS ; BLACK CARBON ; PEANUT HULL ; LEAD ; IMMOBILIZATION ; AMENDMENT
收录类别SCI
语种英语
项目资助者National Major Research Program of China(2013CB934302) ; National Major Research Program of China(2013CB934302) ; National Major Research Program of China(2013CB934302) ; National Major Research Program of China(2013CB934302) ; National Major Research Program of China(2013CB934302) ; National Major Research Program of China(2013CB934302) ; National Major Research Program of China(2013CB934302) ; National Major Research Program of China(2013CB934302) ; National Natural Science Foundation of China(41301347 ; National Natural Science Foundation of China(41301347 ; National Natural Science Foundation of China(41301347 ; National Natural Science Foundation of China(41301347 ; National Natural Science Foundation of China(41301347 ; National Natural Science Foundation of China(41301347 ; National Natural Science Foundation of China(41301347 ; National Natural Science Foundation of China(41301347 ; Anhui Provincial Natural Science Foundation(1408085MKL61) ; Anhui Provincial Natural Science Foundation(1408085MKL61) ; Anhui Provincial Natural Science Foundation(1408085MKL61) ; Anhui Provincial Natural Science Foundation(1408085MKL61) ; Anhui Provincial Natural Science Foundation(1408085MKL61) ; Anhui Provincial Natural Science Foundation(1408085MKL61) ; Anhui Provincial Natural Science Foundation(1408085MKL61) ; Anhui Provincial Natural Science Foundation(1408085MKL61) ; Natural Science Foundation of Anhui Academy of Agricultural Sciences(14A1009) ; Natural Science Foundation of Anhui Academy of Agricultural Sciences(14A1009) ; Natural Science Foundation of Anhui Academy of Agricultural Sciences(14A1009) ; Natural Science Foundation of Anhui Academy of Agricultural Sciences(14A1009) ; Natural Science Foundation of Anhui Academy of Agricultural Sciences(14A1009) ; Natural Science Foundation of Anhui Academy of Agricultural Sciences(14A1009) ; Natural Science Foundation of Anhui Academy of Agricultural Sciences(14A1009) ; Natural Science Foundation of Anhui Academy of Agricultural Sciences(14A1009) ; Scientific and Technical Key Research Program of Auhui ; Scientific and Technical Key Research Program of Auhui ; Scientific and Technical Key Research Program of Auhui ; Scientific and Technical Key Research Program of Auhui ; Scientific and Technical Key Research Program of Auhui ; Scientific and Technical Key Research Program of Auhui ; Scientific and Technical Key Research Program of Auhui ; Scientific and Technical Key Research Program of Auhui ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; CAS/SAFEA International Partnership Program for Creative Research Teams of Chinese Academy of Sciences, China ; 21177132) ; 21177132) ; 21177132) ; 21177132) ; 21177132) ; 21177132) ; 21177132) ; 21177132)
WOS研究方向Engineering ; Environmental Sciences & Ecology
WOS类目Engineering, Environmental ; Engineering, Civil ; Environmental Sciences
WOS记录号WOS:000367699200005
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被引频次:188[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.hfcas.ac.cn:8080/handle/334002/30606
专题中科院固体物理研究所
作者单位1.Chinese Acad Sci, Inst Solid State Phys, Anhui Key Lab Nanomat & Nanotechnol, Key Lab Mat Phys,Ctr Environm & Energy Nanomat, Hefei 230031, Peoples R China
2.Anhui Acad Agr Sci, Inst Soil & Fertilizer, Hefei 230031, Peoples R China
3.Griffith Univ, Ctr Clean Environm & Energy, Nathan, Qld 4222, Australia
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Li, Hongying,Ye, Xinxin,Geng, Zhigang,et al. The influence of biochar type on long-term stabilization for Cd and Cu in contaminated paddy soils[J]. JOURNAL OF HAZARDOUS MATERIALS,2016,304(无):40-48.
APA Li, Hongying.,Ye, Xinxin.,Geng, Zhigang.,Zhou, Hongjian.,Guo, Xisheng.,...&Wang, Guozhong.(2016).The influence of biochar type on long-term stabilization for Cd and Cu in contaminated paddy soils.JOURNAL OF HAZARDOUS MATERIALS,304(无),40-48.
MLA Li, Hongying,et al."The influence of biochar type on long-term stabilization for Cd and Cu in contaminated paddy soils".JOURNAL OF HAZARDOUS MATERIALS 304.无(2016):40-48.
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