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Insights into the reduction of 4-nitrophenol to 4-aminophenol on catalysts
Kong, Xiangkai1,2; Zhu, Hongying3; Chen, ChangLe4; Huang, Guangming3; Chen, Qianwang2,5,6,7
2017-09-16
Source PublicationCHEMICAL PHYSICS LETTERS
Volume684Pages:148-152
AbstractNew insights for the mechanism of nitro to amino groups conversion have been revealed on both N-doped graphene and Ag nanoparticles catalysts, based on the paper assisted ultrasonic spray ionization mass spectrometry: (1) water molecules not NaBH4 are the hydrogen source for the reduced amino groups, (2) NaBH4 could contribute to the ionization of H+ from water, facilitating its adsorption on nitro groups, (3) six different intermediates have been detected to depict the whole catalytic process, and no condensed roots are involved in and (4) this reduction process is spontaneous to some extent, and even without catalysts it is not totally stopped as obtained from the spectral measurements. (C) 2017 Elsevier B.V. All rights reserved.
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences
Funding OrganizationNational Natural Science Foundation of China (NSFC)(21271163 ; National Natural Science Foundation of China (NSFC)(21271163 ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; U1232211 ; U1232211 ; 21374108 ; 21374108 ; 21205111 ; 21205111 ; 51602116) ; 51602116) ; National Natural Science Foundation of China (NSFC)(21271163 ; National Natural Science Foundation of China (NSFC)(21271163 ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; U1232211 ; U1232211 ; 21374108 ; 21374108 ; 21205111 ; 21205111 ; 51602116) ; 51602116)
DOI10.1016/j.cplett.2017.06.049
WOS KeywordAIR-WATER-INTERFACE ; GOLD NANOPARTICLES ; SILVER NANOPARTICLES ; NITRO-COMPOUNDS ; DOPED GRAPHENE ; NITROPHENOL ; NANOCOMPOSITE ; OXIDATION ; EFFICIENT ; RADICALS
Indexed BySCI
Language英语
Funding OrganizationNational Natural Science Foundation of China (NSFC)(21271163 ; National Natural Science Foundation of China (NSFC)(21271163 ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; U1232211 ; U1232211 ; 21374108 ; 21374108 ; 21205111 ; 21205111 ; 51602116) ; 51602116) ; National Natural Science Foundation of China (NSFC)(21271163 ; National Natural Science Foundation of China (NSFC)(21271163 ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; U1232211 ; U1232211 ; 21374108 ; 21374108 ; 21205111 ; 21205111 ; 51602116) ; 51602116)
WOS Research AreaChemistry ; Physics
WOS SubjectChemistry, Physical ; Physics, Atomic, Molecular & Chemical
WOS IDWOS:000407404400024
Citation statistics
Document Type期刊论文
Identifierhttp://ir.hfcas.ac.cn:8080/handle/334002/33574
Collection中科院强磁场科学中心
Affiliation1.Huaibei Normal Univ, Sch Phys & Elect Informat, Huaibei 235000, Peoples R China
2.Chinese Acad Sci, High Magnet Field Lab, Hefei 230031, Anhui, Peoples R China
3.Univ Sci & Technol China, Dept Chem, Hefei 230026, Anhui, Peoples R China
4.Univ Sci & Technol China, Dept Polymer Sci & Engn, Hefei, Anhui, Peoples R China
5.Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China
6.Univ Sci & Technol China, Dept Mat Sci & Engn, Hefei 230026, Anhui, Peoples R China
7.Univ Sci & Technol China, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Hefei 230026, Anhui, Peoples R China
Recommended Citation
GB/T 7714
Kong, Xiangkai,Zhu, Hongying,Chen, ChangLe,et al. Insights into the reduction of 4-nitrophenol to 4-aminophenol on catalysts[J]. CHEMICAL PHYSICS LETTERS,2017,684:148-152.
APA Kong, Xiangkai,Zhu, Hongying,Chen, ChangLe,Huang, Guangming,&Chen, Qianwang.(2017).Insights into the reduction of 4-nitrophenol to 4-aminophenol on catalysts.CHEMICAL PHYSICS LETTERS,684,148-152.
MLA Kong, Xiangkai,et al."Insights into the reduction of 4-nitrophenol to 4-aminophenol on catalysts".CHEMICAL PHYSICS LETTERS 684(2017):148-152.
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