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Insights into the reduction of 4-nitrophenol to 4-aminophenol on catalysts
Kong, Xiangkai1,2; Zhu, Hongying3; Chen, ChangLe4; Huang, Guangming3; Chen, Qianwang2,5,6,7
2017-09-16
发表期刊CHEMICAL PHYSICS LETTERS
卷号684页码:148-152
摘要New insights for the mechanism of nitro to amino groups conversion have been revealed on both N-doped graphene and Ag nanoparticles catalysts, based on the paper assisted ultrasonic spray ionization mass spectrometry: (1) water molecules not NaBH4 are the hydrogen source for the reduced amino groups, (2) NaBH4 could contribute to the ionization of H+ from water, facilitating its adsorption on nitro groups, (3) six different intermediates have been detected to depict the whole catalytic process, and no condensed roots are involved in and (4) this reduction process is spontaneous to some extent, and even without catalysts it is not totally stopped as obtained from the spectral measurements. (C) 2017 Elsevier B.V. All rights reserved.
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
资助者National Natural Science Foundation of China (NSFC)(21271163 ; National Natural Science Foundation of China (NSFC)(21271163 ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; U1232211 ; U1232211 ; 21374108 ; 21374108 ; 21205111 ; 21205111 ; 51602116) ; 51602116) ; National Natural Science Foundation of China (NSFC)(21271163 ; National Natural Science Foundation of China (NSFC)(21271163 ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; U1232211 ; U1232211 ; 21374108 ; 21374108 ; 21205111 ; 21205111 ; 51602116) ; 51602116)
DOI10.1016/j.cplett.2017.06.049
关键词[WOS]AIR-WATER-INTERFACE ; GOLD NANOPARTICLES ; SILVER NANOPARTICLES ; NITRO-COMPOUNDS ; DOPED GRAPHENE ; NITROPHENOL ; NANOCOMPOSITE ; OXIDATION ; EFFICIENT ; RADICALS
收录类别SCI
语种英语
资助者National Natural Science Foundation of China (NSFC)(21271163 ; National Natural Science Foundation of China (NSFC)(21271163 ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; U1232211 ; U1232211 ; 21374108 ; 21374108 ; 21205111 ; 21205111 ; 51602116) ; 51602116) ; National Natural Science Foundation of China (NSFC)(21271163 ; National Natural Science Foundation of China (NSFC)(21271163 ; Anhui Natural Science Foundation(1708085QB40) ; Anhui Natural Science Foundation(1708085QB40) ; U1232211 ; U1232211 ; 21374108 ; 21374108 ; 21205111 ; 21205111 ; 51602116) ; 51602116)
WOS研究方向Chemistry ; Physics
WOS类目Chemistry, Physical ; Physics, Atomic, Molecular & Chemical
WOS记录号WOS:000407404400024
引用统计
文献类型期刊论文
条目标识符http://ir.hfcas.ac.cn:8080/handle/334002/33574
专题中科院强磁场科学中心
作者单位1.Huaibei Normal Univ, Sch Phys & Elect Informat, Huaibei 235000, Peoples R China
2.Chinese Acad Sci, High Magnet Field Lab, Hefei 230031, Anhui, Peoples R China
3.Univ Sci & Technol China, Dept Chem, Hefei 230026, Anhui, Peoples R China
4.Univ Sci & Technol China, Dept Polymer Sci & Engn, Hefei, Anhui, Peoples R China
5.Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China
6.Univ Sci & Technol China, Dept Mat Sci & Engn, Hefei 230026, Anhui, Peoples R China
7.Univ Sci & Technol China, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Hefei 230026, Anhui, Peoples R China
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Kong, Xiangkai,Zhu, Hongying,Chen, ChangLe,et al. Insights into the reduction of 4-nitrophenol to 4-aminophenol on catalysts[J]. CHEMICAL PHYSICS LETTERS,2017,684:148-152.
APA Kong, Xiangkai,Zhu, Hongying,Chen, ChangLe,Huang, Guangming,&Chen, Qianwang.(2017).Insights into the reduction of 4-nitrophenol to 4-aminophenol on catalysts.CHEMICAL PHYSICS LETTERS,684,148-152.
MLA Kong, Xiangkai,et al."Insights into the reduction of 4-nitrophenol to 4-aminophenol on catalysts".CHEMICAL PHYSICS LETTERS 684(2017):148-152.
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