Institutional Repository of Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol,Hefei 230031, Anhui, Peoples R China
Sequential deposition route to efficient Sb2S3 solar cells | |
Zhang, Lijian1; Wu, Chunyan1; Liu, Weifeng1; Yang, Shangfeng1; Wang, Mingtai2; Chen, Tao1; Zhu, Changfei1 | |
2018-11-21 | |
发表期刊 | JOURNAL OF MATERIALS CHEMISTRY A |
ISSN | 2050-7488 |
通讯作者 | Chen, Tao(tchenmse@ustc.edu.cn) ; Zhu, Changfei(cfzhu@ustc.edu.cn) |
摘要 | We report a facile two-step sequential deposition method to prepare Sb2S3 thin films, where antimony acetate and thiourea are utilized as antimony and sulfur sources, respectively. The sequential deposition of two precursor materials followed by swift annealing at mild temperature leads to high-quality Sb2S3 films. The detailed reaction mechanism is revealed on the basis of structural and compositional analyses. By optimizing the concentration of thiourea and annealing temperature, uniform and flat Sb2S3 thin films are obtained with either sulfur-deficiency or sulfur richness. Finally, a planar heterojunction solar cell based on the as-prepared Sb2S3 film delivers a high power conversion efficiency of 5.69%, which is a top value for planar heterojunction Sb2S3 solar cells fabricated by a solution approach. This research provides a convenient and low-cost approach for the deposition of Sb2S3 films for efficient solar cell applications. |
DOI | 10.1039/c8ta08296k |
关键词[WOS] | ATOMIC LAYER DEPOSITION ; THERMAL-DECOMPOSITION ; THIN-FILMS ; THIOUREA ; ABSORBER ; GROWTH |
收录类别 | SCI |
语种 | 英语 |
资助项目 | Recruitment Program of Global Experts (National Natural Science Foundation of China)[GG2060140085] ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology[2016FXZY003] ; Fundamental Research Funds for the Central Universities[WK2060140024] ; Fundamental Research Funds for the Central Universities[CX3430000001] ; Fundamental Research Funds for the Central Universities[WK2060140022] ; Fundamental Research Funds for the Central Universities[WK2060140023] ; Fundamental Research Funds for the Central Universities[WK2060140023] ; Fundamental Research Funds for the Central Universities[WK2060140022] ; Fundamental Research Funds for the Central Universities[CX3430000001] ; Fundamental Research Funds for the Central Universities[WK2060140024] ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology[2016FXZY003] ; Recruitment Program of Global Experts (National Natural Science Foundation of China)[GG2060140085] |
项目资助者 | Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) |
WOS研究方向 | Chemistry ; Energy & Fuels ; Materials Science |
WOS类目 | Chemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary |
WOS记录号 | WOS:000449701900007 |
出版者 | ROYAL SOC CHEMISTRY |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.hfcas.ac.cn:8080/handle/334002/34163 |
专题 | 应用技术研究所 |
通讯作者 | Chen, Tao; Zhu, Changfei |
作者单位 | 1.Univ Sci & Technol China, Dept Mat Sci & Engn, CAS Key Lab Mat Energy Convers, 96 Jinzhai Rd, Hefei 230026, Anhui, Peoples R China 2.Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol, Hefei 230031, Anhui, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Lijian,Wu, Chunyan,Liu, Weifeng,et al. Sequential deposition route to efficient Sb2S3 solar cells[J]. JOURNAL OF MATERIALS CHEMISTRY A,2018,6(43):21320-21326. |
APA | Zhang, Lijian.,Wu, Chunyan.,Liu, Weifeng.,Yang, Shangfeng.,Wang, Mingtai.,...&Zhu, Changfei.(2018).Sequential deposition route to efficient Sb2S3 solar cells.JOURNAL OF MATERIALS CHEMISTRY A,6(43),21320-21326. |
MLA | Zhang, Lijian,et al."Sequential deposition route to efficient Sb2S3 solar cells".JOURNAL OF MATERIALS CHEMISTRY A 6.43(2018):21320-21326. |
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