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Sequential deposition route to efficient Sb2S3 solar cells
Zhang, Lijian1; Wu, Chunyan1; Liu, Weifeng1; Yang, Shangfeng1; Wang, Mingtai2; Chen, Tao1; Zhu, Changfei1
2018-11-21
发表期刊JOURNAL OF MATERIALS CHEMISTRY A
ISSN2050-7488
卷号6期号:43页码:21320-21326
通讯作者Chen, Tao(tchenmse@ustc.edu.cn) ; Zhu, Changfei(cfzhu@ustc.edu.cn)
摘要We report a facile two-step sequential deposition method to prepare Sb2S3 thin films, where antimony acetate and thiourea are utilized as antimony and sulfur sources, respectively. The sequential deposition of two precursor materials followed by swift annealing at mild temperature leads to high-quality Sb2S3 films. The detailed reaction mechanism is revealed on the basis of structural and compositional analyses. By optimizing the concentration of thiourea and annealing temperature, uniform and flat Sb2S3 thin films are obtained with either sulfur-deficiency or sulfur richness. Finally, a planar heterojunction solar cell based on the as-prepared Sb2S3 film delivers a high power conversion efficiency of 5.69%, which is a top value for planar heterojunction Sb2S3 solar cells fabricated by a solution approach. This research provides a convenient and low-cost approach for the deposition of Sb2S3 films for efficient solar cell applications.
资助者Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China)
DOI10.1039/c8ta08296k
关键词[WOS]ATOMIC LAYER DEPOSITION ; THERMAL-DECOMPOSITION ; THIN-FILMS ; THIOUREA ; ABSORBER ; GROWTH
收录类别SCI
语种英语
资助项目Fundamental Research Funds for the Central Universities[WK2060140023] ; Fundamental Research Funds for the Central Universities[WK2060140022] ; Fundamental Research Funds for the Central Universities[CX3430000001] ; Fundamental Research Funds for the Central Universities[WK2060140024] ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology[2016FXZY003] ; Recruitment Program of Global Experts (National Natural Science Foundation of China)[GG2060140085]
资助者Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Major/Innovative Program of Development Foundation of Hefei Center for Physical Science and Technology ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China) ; Recruitment Program of Global Experts (National Natural Science Foundation of China)
WOS研究方向Chemistry ; Energy & Fuels ; Materials Science
WOS类目Chemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary
WOS记录号WOS:000449701900007
出版者ROYAL SOC CHEMISTRY
引用统计
被引频次:1[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.hfcas.ac.cn:8080/handle/334002/34164
专题应用技术研究所
通讯作者Chen, Tao; Zhu, Changfei
作者单位1.Univ Sci & Technol China, Dept Mat Sci & Engn, CAS Key Lab Mat Energy Convers, 96 Jinzhai Rd, Hefei 230026, Anhui, Peoples R China
2.Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol, Hefei 230031, Anhui, Peoples R China
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Zhang, Lijian,Wu, Chunyan,Liu, Weifeng,et al. Sequential deposition route to efficient Sb2S3 solar cells[J]. JOURNAL OF MATERIALS CHEMISTRY A,2018,6(43):21320-21326.
APA Zhang, Lijian.,Wu, Chunyan.,Liu, Weifeng.,Yang, Shangfeng.,Wang, Mingtai.,...&Zhu, Changfei.(2018).Sequential deposition route to efficient Sb2S3 solar cells.JOURNAL OF MATERIALS CHEMISTRY A,6(43),21320-21326.
MLA Zhang, Lijian,et al."Sequential deposition route to efficient Sb2S3 solar cells".JOURNAL OF MATERIALS CHEMISTRY A 6.43(2018):21320-21326.
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