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NH4I Facilitated the Formation of Mixed-Dimensional Perovskite and Improved Stability at Different Annealing Temperatures
Zheng, Haiying1,2; Liu, Guozhen1,2; Xu, Xiaoxiao1,2; Zhang, Xianxi3; Alsaedi, Ahmed4; Hayat, Tasawar4,5; Pan, Xu1
2018-11-05
发表期刊ACS SUSTAINABLE CHEMISTRY & ENGINEERING
ISSN2168-0485
卷号6期号:11页码:15143-15150
通讯作者Pan, Xu(xpan@rntek.cas.cn)
摘要Hybrid organic/inorganic perovskites as light absorption layer have received considerable attention because of their preeminent photovoltaic performance. Presently, gaining high power conversion efficiency (PCE) and longterm stability of perovskite solar cells (PSCs) is very crucial to achieve their practical application. Here, NH4I was introduced to fabricate the mixed dimensional (MD) perovskite films at different annealing temperatures. The addition of NH4I could improve the preferential crystal orientation within the polycrystalline, favor the formation of MD perovskite, and suppress the existence of yellow PbI2 phase. The results indicate that MD perovskite films have a smoother surface, preferentially oriented perovskite crystal, and better optical properties at the same annealing temperature, compared with formamidinium (FA) perovskite. The MD perovskite device displays excellent photovoltaic performance possessing a high PCE of 18.93% at 100 degrees C. More importantly, the 1200 h humidity and 200 h heat stability tests reveal that the MD perovskite devices at optimized annealing temperature show great stability against moisture and heat. The findings are crucial to perovskite photovoltaics on improving the PCE and the long-term stability in industrialization and other applications.
关键词NH4I Mixed dimensional perovskite Annealing temperature High efficiency Long-term stability
资助者STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China
DOI10.1021/acssuschemeng.8b03604
关键词[WOS]SOLAR-CELLS ; HIGH-PERFORMANCE ; THIN-FILMS ; DEGRADATION ; EXCHANGE ; FABRICATION ; LAYERS
收录类别SCI
语种英语
资助项目STS project of Chinese Academy of Sciences[KFJ-SW-STS-152] ; National High Technology Research and Development Program of China[2015AA050602]
资助者STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; STS project of Chinese Academy of Sciences ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China ; National High Technology Research and Development Program of China
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Engineering
WOS类目Chemistry, Multidisciplinary ; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY ; Engineering, Chemical
WOS记录号WOS:000449577200167
出版者AMER CHEMICAL SOC
引用统计
文献类型期刊论文
条目标识符http://ir.hfcas.ac.cn:8080/handle/334002/34326
专题应用技术研究所
通讯作者Pan, Xu
作者单位1.Chinese Acad Sci, Hefei Inst Phys Sci, Inst Appl Technol, Key Lab Photovolta & Energy Conservat Mat, 2221 Changjiangxi Rd, Hefei 230088, Anhui, Peoples R China
2.Univ Sci & Technol China, 96 Jinzhai Rd, Hefei 230026, Anhui, Peoples R China
3.Liaocheng Univ, Collaborat Innovat Ctr Chem Energy Storage & Nove, Shandong Prov Key Lab, Hunan 1 Rd, Liaocheng 252000, Shandong, Peoples R China
4.King Abdulaziz Univ, Fac Sci, Dept Math, NAAM Res Grp, Jeddah 21589, Saudi Arabia
5.Quaid I Azam Univ, Dept Math, Islamabad 44000, Pakistan
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GB/T 7714
Zheng, Haiying,Liu, Guozhen,Xu, Xiaoxiao,et al. NH4I Facilitated the Formation of Mixed-Dimensional Perovskite and Improved Stability at Different Annealing Temperatures[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2018,6(11):15143-15150.
APA Zheng, Haiying.,Liu, Guozhen.,Xu, Xiaoxiao.,Zhang, Xianxi.,Alsaedi, Ahmed.,...&Pan, Xu.(2018).NH4I Facilitated the Formation of Mixed-Dimensional Perovskite and Improved Stability at Different Annealing Temperatures.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,6(11),15143-15150.
MLA Zheng, Haiying,et al."NH4I Facilitated the Formation of Mixed-Dimensional Perovskite and Improved Stability at Different Annealing Temperatures".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 6.11(2018):15143-15150.
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