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Spin-induced multiferroicity in the binary perovskite manganite Mn2O3
Cong, Junzhuang1; Zhai, Kun1; Chai, Yisheng1; Shang, Dashan1; Khalyavin, Dmitry D.2; Johnson, Roger D.3; Kozlenko, Denis P.4; Kichanov, Sergey E.4; Abakumov, Artem M.5; Tsirlin, Alexander A.6; Dubrovinsky, Leonid7; Xu, Xueli8; Sheng, Zhigao8; Ovsyannikov, Sergey, V7,9; Sun, Young1,10
2018-07-31
发表期刊NATURE COMMUNICATIONS
ISSN2041-1723
通讯作者Ovsyannikov, Sergey, V(sergey.ovsyannikov@uni-bayreuth.de) ; Sun, Young(youngsun@iphy.ac.cn)
摘要The ABO(3) perovskite oxides exhibit a wide range of interesting physical phenomena remaining in the focus of extensive scientific investigations and various industrial applications. In order to form a perovskite structure, the cations occupying the A and B positions in the lattice, as a rule, should be different. Nevertheless, the unique binary perovskite manganite Mn2O3 containing the same element in both A and B positions can be synthesized under high-pressure high-temperature conditions. Here, we show that this material exhibits magnetically driven ferroelectricity and a pronounced magnetoelectric effect at low temperatures. Neutron powder diffraction revealed two intricate antiferromagnetic structures below 100 K, driven by a strong interplay between spin, charge, and orbital degrees of freedom. The peculiar multiferroicity in the Mn2O3 perovskite is ascribed to a combined effect involving several mechanisms. Our work demonstrates the potential of binary perovskite oxides for creating materials with highly promising electric and magnetic properties.
DOI10.1038/s41467-018-05296-0
关键词[WOS]THIN-FILMS ; OXIDE ; CHARGE ; HETEROSTRUCTURES ; POLARIZATION ; TRANSITION ; CDMN7O12 ; PHYSICS
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China[11534015] ; National Natural Science Foundation of China[51725104] ; National Key Research and Development Programm of China[2016YFA0300701] ; Chinese Academy of Sciences[XDB07030200] ; Deutsche Forschungsgemeinschaft (DFG)[OV-110/1-3] ; National Natural Science Foundation of China[11534015] ; National Natural Science Foundation of China[51725104] ; National Key Research and Development Programm of China[2016YFA0300701] ; Chinese Academy of Sciences[XDB07030200] ; Deutsche Forschungsgemeinschaft (DFG)[OV-110/1-3]
项目资助者National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; National Key Research and Development Programm of China ; 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Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG) ; Deutsche Forschungsgemeinschaft (DFG)
WOS研究方向Science & Technology - Other Topics
WOS类目Multidisciplinary Sciences
WOS记录号WOS:000440280700001
出版者NATURE PUBLISHING GROUP
引用统计
被引频次：32[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.hfcas.ac.cn:8080/handle/334002/37697
专题中科院强磁场科学中心
通讯作者Ovsyannikov, Sergey, V; Sun, Young
作者单位1.Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China
2.Rutherford Appleton Lab STFC, ISIS Facil, Didcot OX11 0QX, Oxon, England
3.Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England
4.Joint Inst Nucl Res, Frank Lab Neutron Phys, Dubna 141980, Russia
5.Skolkovo Inst Sci & Technol, Ctr Electrochem Energy Storage, Nobel St 3, Moscow 143026, Russia
6.Univ Augsburg, Ctr Elect Correlat & Magnetism, Inst Phys, Expt Phys 6, D-86135 Augsburg, Germany
7.Univ Bayreuth, Bayer Geoinst, Univ Str 30, D-95447 Bayreuth, Germany
8.Chinese Acad Sci, High Magnet Field Lab, Hefei 230031, Anhui, Peoples R China
9.Russian Acad Sci, Urals Div, Inst Solid State Chem, 91 Pervomayskaya Str, Ekaterinburg 620990, Russia
10.Univ Chinese Acad Sci, Sch Phys Sci, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714		 Cong, Junzhuang,Zhai, Kun,Chai, Yisheng,et al. Spin-induced multiferroicity in the binary perovskite manganite Mn2O3[J]. NATURE COMMUNICATIONS,2018,9:7.
APA Cong, Junzhuang.,Zhai, Kun.,Chai, Yisheng.,Shang, Dashan.,Khalyavin, Dmitry D..,...&Sun, Young.(2018).Spin-induced multiferroicity in the binary perovskite manganite Mn2O3.NATURE COMMUNICATIONS,9,7.
MLA Cong, Junzhuang,et al."Spin-induced multiferroicity in the binary perovskite manganite Mn2O3".NATURE COMMUNICATIONS 9(2018):7.
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